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2 article(s) from Hameau, Aurélien

Fluorescent phosphorus dendrimers excited by two photons: synthesis, two-photon absorption properties and biological uses

Anne-Marie Caminade,
Artem Zibarov,
Eduardo Cueto Diaz,
Aurélien Hameau,
Maxime Klausen,
Kathleen Moineau-Chane Ching,
Jean-Pierre Majoral,
Jean-Baptiste Verlhac,
Olivier Mongin and
Mireille Blanchard-Desce

Beilstein J. Org. Chem. 2019, 15, 2287–2303, doi:10.3762/bjoc.15.221

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Graphical Abstract

Figure 1: Jablonski-type diagram displaying the classical one-photon excited fluorescence (left), and the les...

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Figure 2: Two ways to represent schematized structures of dendrimers, showing the different generations (laye...

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Scheme 1: Synthesis of phosphorhydrazone dendrimers, from the core to generation 2. Generation 1 dendrimers w...

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Scheme 2: Full structure of the generation 1 dendrimer bearing 12 blue-emitting TPA fluorophores on the surfa...

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Figure 3: Linear structure of the generation 2 dendrimer bearing 24 green-emitting TPA fluorophores on the su...

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Scheme 3: Synthesis of the dioxaborine-functionalized dendrimer of generation 4.

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Figure 4: Diverse structures of multistilbazole compounds, and graph of the σ₂^max/ε^max response, depending on...

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Figure 5: Nile Red derivatives: monomer (M) and two generations of dendrimers.

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Scheme 4: Dumbbell-like dendrimers (third generation) having one TPA fluorophore at the core, and ammonium te...

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Scheme 5: Another example of dumbbell-like dendrimers having one TPA fluorophore at the core, and P(S)Cl₂ or ...

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Scheme 6: The 12 steps needed to synthesize a sophisticated TPA fluorophore, to be used as branches of dendri...

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Scheme 7: Synthesis of dendrimers having TPA fluorophores as branches and water-solubilizing functions on the...

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Figure 6: Other types of dendrimers having TPA fluorophores as branches and water-solubilizing functions on t...

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Figure 7: Generations 0, 1, and 2 of dumbbell-like dendrimers having one fluorophore at the core and either 1...

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Figure 8: Double layer fluorescent dendrimer.

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Figure 9: Dumbbell-like dendrimer used for two-photon imaging of the blood vessels of a living rat olfactory ...

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Figure 10: Fluorescent gold complex having high antiproliferative activities against different tumor cell line...

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Figure 11: A fluorescent water-soluble dendrimer, applicable for two-photon photodynamic therapy and imaging.

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Figure 12: Schematization of the different types of TPA fluorescent phosphorus dendrimers and dendritic struct...

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Review

Published 24 Sep 2019

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Synthesis of dye/fluorescent functionalized dendrons based on cyclotriphosphazene

Aurélien Hameau,
Sabine Fuchs,
Régis Laurent,
Jean-Pierre Majoral and
Anne-Marie Caminade

Beilstein J. Org. Chem. 2011, 7, 1577–1583, doi:10.3762/bjoc.7.186

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Scheme 1: Synthesis of functionalized phenols. Reagents and conditions: a) Boc₂O, 1.0 equiv, THF, 0 °C → rt, ...

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Scheme 2: Single substitution of hexachlorocyclotriphosphazene. Reagents and conditions: a) Cs₂CO₃, 1.67 equi...

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Scheme 3: Synthesis of dansylated dendrons. Reagents and conditions: a) Cs₂CO₃, 11 equiv, THF, rt, 48 h. b) Cs...

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Scheme 4: Synthesis of dabsylated dendrons. Reagents and conditions: a) Cs₂CO₃, 11 equiv, THF, rt, 48 h. b) T...

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Figure 1: UV–vis spectra of compounds 8–10.

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Figure 2: UV–vis spectra of compounds 4, 11 and 12 in dioxane.

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Figure 3: Excitation (left) and emission (right) spectra of compounds 8–10 in 1,4-dioxane (the excitation spe...

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Figure 4: Emission spectra (λ_exc = 347 nm) of compound 10 in mixtures water/dioxane with different molar frac...

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Figure 5: λ_em,max of 10 in mixture water/dioxane vs molar fraction of water in dioxane (filled squares) and v...

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Full Research Paper

Published 28 Nov 2011

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